Devious Journal Entry

Robotech (kind of cheating, I know)
Macross
Galaxy Express 999
Mysterious Cities of Gold
Grimm's Fairy Tales
Future Boy Conan
Fist of the North Star (some)
Space Battleship Yamato
Voltron (some)
Speed Racer (some)
Astro-Boy (some)
Urusei Yatsura
Battle Angel Alita
Cat's Eye (some)
Sailor Moon (some)
DBZ (very few)
DearS
Onegai Sensei
Fruitsbasket
Full Metal Alchemist
Full Metal Alchemist Brotherhood
Last Exile
Last Exile Fam The Silver Wing
Bakuretsu Tenshi
Love Hina
Getbackers
Monster
Kyogoku's Hundred Ghost Stories
Lain
Helsing
Gantz
Elfen Lied
Girls Bravo
Aishiteruze Baby
Bleach (through Bontou storyline)
Naruto (first 26 episodes)
One Piece (first 26 episodes)
Gunslinger Girl 1, 2
Genshiken 1, 2, 3
Tiger and Bunny
Cowboy Bebop
Blue Gender
Trigun
Gun X Sword
Silver Spoon 1, 2
Paranoia Agent
Kino's Journey
Sword Art Online 1, 2 (in progress)
FLCL
Space Dandy (in progress)
Samurai Champloo
Ichigo 100%
Ghost in the Shell Stand Alone Complex
Ghost in the Shell 2nd Gig
.Hack/Sign
Death Note
Read or Die
Haibane Renmei
Ranma 1/2
Kimagure Orange Road
Baccano!
Victorian Romance Emma
Shuffle 1, 2 (aka Shuffle Memories)
Gilgamesh
Azumanga Daioh
The Melancholy of Haruhi Suzumiya 1, 2
Honey and Clover
Gungrave
Gankutsuo (Count of Monte Cristo)
Evangelion
Toward the Terra
Narutaru
Rosario + Vampire
12 Kingdoms
Planetes
Witch Hunter Robin
Chi's Sweet Home
Dogtato-kun
Ocha-Ken
Tokyo Magnitude 8.0
Speed Grapher
Chobits
sCRYed
Yakitate Ja-pan!
Gundam Wing
Darker Than Black
Inuyasha
Air
Gundam Seed (some)
Berserk
Attack on Titan
Soul Eater 1, and that spin off series with N.O.T.
Great Teacher Onizuka
Excel Saga
Lupin III
Lupin III, Woman Called Fujiko
Pumpkin Scissors
Mysterious Girlfriend X
Midori no Hibe
High School of the Dead
Daughter of Twenty Faces
Fairy Tale
Desert Punk
Ah Megami-sama!
Black Jack
Midori no Hibe
Welcome to the NHK
Gallery Fake
Shakugan no Shana
Eureka 7
Tide Line Blue
Grenadier
Windy Tales
Samurai 7
Initial D
King Jing of Bandits
Popotan
Ninja Scroll The Series
Eden of the East
Wolf's Rain
Big O
Astro Boy 2003
Tokyo Underground
Gakko no Kaidan
Denno Coil
Trinity Blood
Weiss Kreuz
Great Teacher Onizuka
Tsukuyomi Moon Phase
Occult Academy
Escaflowne
Full Metal Panic
Gargantia on the Verdurous Planet
Knights of Sidonia
Kamichu
Kill La Kill
Mushishi

MOVIES --

ALL Studio Ghibli films (minus Princes Kaguya and When Marnie Was There)
ALL Satoshi Kon films
Demon City Shinjuku
Ninja Scroll
Voices of a Distant Star
Beyond the Clouds: Place Promised to Us in Our Early Days
5 Centimeters Per Second
Wicked City
Akira
Steamboy
Vampire Hunter D
FMA: Conquerer of Shambalah
UY: Beautiful Dreamer
Golgo 13 - The Professional
Galaxy Express 999 (Bonjour and Adieu)
Neo Tokyo
City Hunter
Armitage III
Kimba The White Lion
Cowboy Bebop Movie
Princess Arete
Animatrix
Ghost in the Shell 1, 2
Final Fantasy VII: Advent Children
The Girl Who Leapt Through Time
And... All those damn Evangelion movies
ERASED
One-Punch Man
FLCL

IN PROGRESS --
Space Dandy
Sword Art Online 2
Tokyo Ghoul
Zankyou no Terror
Blood Lad
Rage of Bahamut (Ep. 2 -- debating whether to finish)
Log Horizon (Started Ep. 1, will finish after SAO2)
JoJo's Bizarre Adventure (Episode 1 -- may replace Bahamut)
Stella Women's Academy High School Division Class C3
Parasyte

Some of my favorite shows are Cowboy Bebop, Trigun, the original Full Metal Alchemist, Evangelion, Death Note, Last Exile, Sword Art Online, Ghost in the Shell Stand Alone Complex, Kino's Journey, Gunslinger Girl, Tiger and Bunny, Macross, Welcome to the NHK, Elfen Lied, Melancholy of Suzumiya, Monster, Paranoia Agent...

It's hard to say what's the best, but Cowboy Bebop is still my favorite.... even though it's almost cliche to say that.

As for movies, that's too tough. I am a huge of fan of Satoshi Kon, though. And Miyazaki, obviously.

For years, I keep getting asked what my Top 5 Anime Series are.
Well, I can give you My Top 3 --
1. COWBOY BEBOP
2. TRIGUN
3. FULL METAL ALCHEMIST (2003)*
Those three haven't really changed in years. So I'm comfortable saying those are my final answers.
The remaining two slots are completely dependent on my mood and subject to change. But I can guarantee these shows will always be in the lineup for 4. and 5.
Most often--?
PARANOIA AGENT
EVANGELION
Other picks--?
CAPTAIN HARLOCK (1978)
KINO'S JOURNEY
GURREN LAGANN**
MACROSS
DEATH NOTE
MUSHISHI
TOKYO MAGNITUDE 8.0
FUTURE BOY CONAN
AZUMANGA DAIOH
MONSTER
WOLF'S RAIN
WELCOME TO THE NHK
MADOKA MAGICA
ELFEN LIED
THE TWELVE KINGDOMS
LAST EXILE
TIGER AND BUNNY
GUNSLINGER GIRL
GHOST IN THE SHELL STAND ALONE COMPLEX
LUPIN III
Of course, there's a ton of other shows I love.
But those tend to always show up first when I'm thinking of favorite anime.
__________________
* = No, I don't hate FMA Brotherhood. I just prefer the '03 series more.
** = I also love FLCL. But it's so short. It's less of a series to me, and more of an OVA. LAGANN kind of takes its spot because of that.

100Josie and the Pussycats

99MASK

98Clerks : The Animated Series

97The Smurfs

96Star Trek: The Animated Series

95Fullmetal Alchemist

94The Boondocks

93Darkwing Duck

92Rugrats

91Harvey Birdman, Attorney at Law

90Afro Samurai

89Star Wars: The Clone Wars

88Woody Woodpecker

87Frisky Dingo

86Astro Boy

85Foster's Home for Imaginary Friends

84Spider-Man (1994 TV series)

83Teen Titans

82Fat Albert and the Cosby Kids

81TaleSpin

80Alvin and the Chipmunks

79Sealab 2021

78Dragon Ball Z

77Johnny Quest

76Voltron

75Dr. Katz, Professional Therapist

74Underdog

73Mobile Suit Gundam Wing

72Dexter's Labratory

71Johnny Bravo

69Mighty Mouse

68Popeye

67The Pink Panther Show

66Tom And Jerry

65Todd McFarlane's Spawn

64Dungeons & Dragons

63Huckleberry Hound

Chip 'N Dale: Rescue Rangers
59
Spider-Man and His Amazing Friends
58
He-Man and the Masters of the Universe
57
Invader Zim
56
Venture Brothers
55
Teenage Mutant Ninja Turtles
54
Inspector Gadget
53
Freakazoid
52
Galaxy High
51
Death Note
50
Super Friends
49
ThunderCats
48
Duckman
47
Pinky and The Brain
46
The Jetsons
45
Gargoyles
44
Battle of the Planets
43
Samurai Jack
42
The Powerpuff Girls
41
Tiny Toon Adventures
40
Batman Beyond
39
Aqua Teen Hunger Force
38
Naruto
37
Space Ghost Coast to Coast
36
Superman: The Animated Series
35
Avatar: The Last Airbender
34
Robotech
33
Schoolhouse Rock!
32
Liquid Television
31
Muppet Babies
30
The Spectacular Spider-Man
29
Speed Racer
28
Home Movies
27
King of the Hill
26
The Critic
25
Robot Chicken
24
Scooby-Doo, Where Are You!
23
Transformers
22
The Real Ghostbusters
21
Star Wars: Clone Wars (2003 TV series)
20
Justice League Unlimited
19
G.I. Joe
18
Duck Tales
17
Animaniacs
16
The Maxx
15
SpongeBob SquarePants
14
Cowboy Bebop
13
X-Men
12
Ren and Stimpy
11
Rocky and Bullwinkle
10
Neon Genesis Evangelion
09
The Flintstones
08
Futurama

The Tick
05
Beavis and Butt-Head
04
South Park
03
Looney Tunes
02
Batman: The Animated Series
01
The Simpsons